Research

Manganites


We have shown with angle-resolved photoemission spectroscopy (ARPES) that the electronic structure in the ferromagnetic metallic (FM) groundstate of the colossal magnetoresistive (CMR) bilayer manganite La1.2Sr1.8Mn2O7 (LSMO) shows striking similarities to that of the pseudogap phase in heavily underdoped cuprates high temperature superconductors (HTSC). The FM phase is a polaronic metal, albeit with a strong anisotropic distribution of spectral weight in momentum space exhibiting a nodal–antinodal dichotomy. Quasiparticle excitations (QP) have been detected for the first time along the nodal direction (i.e. diagonal), and they are found to determine the metallic transport properties in the FM phase. Since this nodal-antinodal dichotomy in momentum space was so far considered a characteristically unique feature of the copper oxide HTSC, these findings cast doubt on the assumption that the pseudogap state and the nodal-antinodal dichotomy in the copper oxides HTSC are hallmarks of the superconductivity state. Furthermore, we found that the temperature dependent evolution of the nodal QP in LSMO tracks remarkably well the DC conductivity, thus accounting for the macroscopic transport properties in LSMO. Our results indicate that the microscopic mechanism leading to the CMR effect in manganites is intrinsically a quantum phase transition which is kinetic energy driven and linked to a crossover from a small polaron hopping regime in the paramagnetic state to a coherent polaronic conductor in the FM state.